Vibrational sum-frequency generation (VSFG) is a nonlinear spectroscopic method widely used to investigate the molecular structure and dynamics of surface systems. However, in far-field observations, ...
We present a microscopic description of the vibrational spectroscopy of the OH stretch of HOD in liquid D 2 O. Our model predicts that OH frequency correlations decay with a sharp and rapid (≈35 fs) ...
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